Technique developed for rapid screening of new types of solar cells

MIT researchers and other institutions have come up with a way to bypass such expensive and time-consuming fabrication and testing for solar panels and cells, allowing for a rapid screening of far more variations than would be practical through the traditional approach.

01/19/2018


This experimental setup was used by the team to measure the electrical output of a sample of solar cell material, under controlled conditions of varying temperature and illumination. Courtesy: Riley Brandt, MITFinding better, more efficient materials for future solar panels is usually a slow and painstaking process. Researchers typically must produce lab samples—which are often composed of multiple layers of different materials bonded together—for extensive testing.

Now, a team at MIT and other institutions has come up with a way to bypass such expensive and time-consuming fabrication and testing, allowing for a rapid screening of far more variations than would be practical through the traditional approach.

The process could not only speed up the search for new formulations, but also do a more accurate job of predicting their performance, explained Rachel Kurchin, an MIT graduate student and co-author of a paper describing the new process that appears in the journal Joule. Traditional methods, she said, "often require you to make a specialized sample, but that differs from an actual cell and may not be fully representative" of a real solar cell's performance.

For example, typical testing methods show the behavior of the "majority carriers," the predominant particles or vacancies whose movement produces an electric current through a material. But in the case of photovoltaic (PV) materials, Kurchin explained, it is actually the minority carriers—those far less abundant in the material—that are the limiting factor in a device's overall efficiency, and those are much more difficult to measure. In addition, typical procedures only measure the flow of current in one set of directions—within the plane of a thin-film material - whereas it's up-down flow that is actually harnessed in a working solar cell. In many materials, that flow can be "drastically different," making it critical to understand in order to properly characterize the material, she says.

"Historically, the rate of new materials development is slow - typically 10 to 25 years," said Tonio Buonassisi, an associate professor of mechanical engineering at MIT and senior author of the paper. "One of the things that makes the process slow is the long time it takes to troubleshoot early-stage prototype devices," he says. "Performing characterization takes time - sometimes weeks or months - and the measurements do not always have the necessary sensitivity to determine the root cause of any problems."

So, Buonassisi said, "The bottom line is, if we want to accelerate the pace of new materials development, it is imperative that we figure out faster and more accurate ways to troubleshoot our early-stage materials and prototype devices." And that's what the team has now accomplished. They have developed a set of tools that can be used to make accurate, rapid assessments of proposed materials, using a series of relatively simple lab tests combined with computer modeling of the physical properties of the material itself, as well as additional modeling based on a statistical method known as Bayesian inference.

The system involves making a simple test device, then measuring its current output under different levels of illumination and different voltages, to quantify exactly how the performance varies under these changing conditions. These values are then used to refine the statistical model.

"After we acquire many current-voltage measurements [of the sample] at different temperatures and illumination intensities, we need to figure out what combination of materials and interface variables make the best fit with our set of measurements," Buonassisi said. "Representing each parameter as a probability distribution allows us to account for experimental uncertainty, and it also allows us to suss out which parameters are covarying."

The Bayesian inference process allows the estimates of each parameter to be updated based on each new measurement, gradually refining the estimates and homing in ever closer to the precise answer, he says.

In seeking a combination of materials for a particular kind of application, Kurchin said, "We put in all these materials properties and interface properties, and it will tell you what the output will look like."

Kurchin said the system is simple enough that, even for materials that have been less well-characterized in the lab. "We're still able to run this without tremendous computer overhead." Making use of the computational tools to screen possible materials will be increasingly useful because "lab equipment has gotten more expensive, and computers have gotten cheaper. This method allows you to minimize your use of complicated lab equipment."

The basic methodology, Buonassisi said, could be applied to a wide variety of different materials evaluations, not just solar cells—in fact, it may apply to any system that involves a computer model for the output of an experimental measurement. "For example, this approach excels in figuring out which material or interface property might be limiting performance, even for complex stacks of materials like batteries, thermoelectric devices, or composites used in tennis shoes or airplane wings. It is especially useful for early-stage research, where many things might be going wrong at once."

Going forward, he said, "Our vision is to link up this fast characterization method with the faster materials and device synthesis methods we've developed in our lab." Ultimately, he said, "I'm very hopeful the combination of high-throughput computing, automation, and machine learning will help us accelerate the rate of novel materials development by more than a factor of five. This could be transformative, bringing the timelines for new materials-science discoveries down from 20 years to about three to five years."

Massachusetts Institute of Technology

www.mit.edu 

- Edited by Chris Vavra, production editor, Control Engineering, CFE Media, cvavra@cfemedia.com. See more Control Engineering energy and power stories.



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